石油化工高等学校学报 ›› 2023, Vol. 36 ›› Issue (4): 1-12.DOI: 10.12422/j.issn.1006-396X.2023.04.001

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CO2RR稀土基催化剂的研究进展

刘嘉敏(), 越婷婷, 常迎, 郭少红, 贾晶春(), 贾美林   

  1. 内蒙古师范大学 化学与环境科学学院,内蒙古 呼和浩特 010022
  • 收稿日期:2022-09-05 修回日期:2022-12-05 出版日期:2023-08-25 发布日期:2023-09-05
  • 通讯作者: 贾晶春
  • 作者简介:刘嘉敏(1997⁃),女,硕士研究生,从事电化学方面的研究;E⁃mail:1670881314@qq.com
  • 基金资助:
    内蒙古自治区科技计划项目(2020PT0003);内蒙古自然科学基金青年项目(2022QN02002);内蒙古师范大学高层引进人才启动基金项目(2018YJRC001)

Research Progress on Rare Earth⁃Based Catalysts for CO2 Reduction Reaction(CO2RR)

Jiamin Liu(), Tingting Yue, Ying Chang, Shaohong Guo, Jingchun Jia(), Meilin Jia   

  1. College of Chemistry and Environmental Science,Inner Mongolia Normal University,Hohhot Inner Mongolia 010022,China
  • Received:2022-09-05 Revised:2022-12-05 Published:2023-08-25 Online:2023-09-05
  • Contact: Jingchun Jia

摘要:

化石燃料的大规模使用导致CO2过度排放,造成气温升高、冰川融化、病虫害加剧等一系列问题。通过电化学还原CO2(CO2RR)将CO2转化为有价值的化学品和燃料,已成为实现碳循环的一种途径。多年来,已将金属及其氧化物、碳基材料、单原子催化剂等不同电催化剂用于CO2RR并取得了一定的进展,但作为“工业维生素”的稀土元素用于CO2RR的报道较少。综述了稀土元素作为载体、主催化剂、助催化剂用于CO2RR的情况,探究了稀土元素材料在CO2RR中的催化性能,以期促进对工业应用的研究。

关键词: 主催化剂, 助催化剂, 载体, CO2还原, 二氧化铈, 催化剂

Abstract:

The large?scale use of fossil fuels has led to excessive CO2 emissions, resulting in a series of problems such as rising temperatures, melting glaciers, and the accumulation of diseases and pests. Using electrochemical reduction of CO2 (CO2RR) to convert CO2 into valuable chemicals and fuels has become a way to realize the carbon cycle. Over the years, good progress has been made in using metals and their oxides, carbon based materials, monatomic catalysts and other electrocatalysts for CO2RR, but rare earth metals as "industrial vitamins" have been rarely reported for CO2RR. This paper summarizes the application of rare earth elements as carriers, main catalysts and cocatalysts in CO2RR, and explores the catalytic performance of rare earth materials in CO2RR, so as to promote practical research of industrial application.

Key words: Main catalyst, Cocatalyst, Support, CO2 reduction, Cerium dioxide, Catalyst

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引用本文

刘嘉敏, 越婷婷, 常迎, 郭少红, 贾晶春, 贾美林. CO2RR稀土基催化剂的研究进展[J]. 石油化工高等学校学报, 2023, 36(4): 1-12.

Jiamin Liu, Tingting Yue, Ying Chang, Shaohong Guo, Jingchun Jia, Meilin Jia. Research Progress on Rare Earth⁃Based Catalysts for CO2 Reduction Reaction(CO2RR)[J]. Journal of Petrochemical Universities, 2023, 36(4): 1-12.

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