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Preparation and Properties of Fully Biodegradable High Impact PLA/PBAT Composites
Wenxin JIANG, Guangxiang ZHANG, Ke YANG, Guiyan ZHAO
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Poly (butyleneadipate-co-terephthalate) (PBAT) was used to toughen poly (lactic acid) (PLA), and a fully biodegradable high impact PLA/PBAT composite was prepared. To improve the interface compatibility between PBAT and PLA, PBAT grafted glycidyl methacrylate (GMA)(PBAT-GMA) compatibilizer was prepared by the melt grafting method. The effect of the mass fraction of compatibilizer on the properties of PLA/PBAT composite was studied. The results show that with the increase of PBAT-GMA mass fraction, the impact strength of the composites is significantly improved. When the PBAT?GMA mass fraction is 30%, the impact strength of the composites reaches 64.8 kJ/m2, and the elongation at break is 289.9%; the compatibilizing mechanism is the epoxy groups on PBAT?GMA can react with the end groups of PLA, which effectively improves the interfacial compatibility between PLA and PBAT.

2024, 44 (5): 31-37. DOI: 10.12422/j.issn.1672-6952.2024.05.005